Hole-Transporting Materials Based on Twisted Bimesitylenes for Stable Perovskite Solar Cells with High Efficiency

Yan Duo Lin; Bo Yu Ke; Kun Mu Lee; Sheng Hsiung Chang; Kai Hung Wang; Shih Han Huang; Chun Guey Wu; Po Ting Chou; Samik Jhulki; Jarugu Narasimha Moorthy; Yuan Jay Chang; Kang Ling Liau; Hsin Cheng Chung; Ching Yang Liu; Shih Sheng Sun; Tahsin J. Chow

doi:10.1002/cssc.201501392

Hole-Transporting Materials Based on Twisted Bimesitylenes for Stable Perovskite Solar Cells with High Efficiency

Yan Duo Lin
, Bo Yu Ke
, Kun Mu Lee
, Sheng Hsiung Chang
, Kai Hung Wang
, Shih Han Huang
, Chun Guey Wu
, Po Ting Chou
, Samik Jhulki
, Jarugu Narasimha Moorthy
, Yuan Jay Chang
, Kang Ling Liau
, Hsin Cheng Chung
, Ching Yang Liu
, Shih Sheng Sun
, Tahsin J. Chow^*

^*Corresponding author for this work

Academia Sinica - Institute of Chemistry
National Central University
Indian Institute of Technology Kanpur
Tunghai University
Chinese Culture University

Research output: Contribution to journal › Journal Article › peer-review

50 Scopus citations

Abstract

A new class of hole-transport materials (HTMs) based on the bimesitylene core designed for mesoporous perovskite solar cells is introduced. Devices fabricated using two of these derivatives yield higher open-circuit voltage values than the commonly used spiro-OMeTAD. Power conversion efficiency (PCE) values of up to 12.11 % are obtained in perovskite-based devices using these new HTMs. The stability of the device made using the highest performing HTM (P1) is improved compared with spiro-OMeTAD as evidenced through long-term stability tests over 1000h.

Original language	English
Pages (from-to)	274-279
Number of pages	6
Journal	ChemSusChem
Volume	9
Issue number	3
DOIs	https://doi.org/10.1002/cssc.201501392
State	Published - 08 02 2016
Externally published	Yes

Bibliographical note

Publisher Copyright:
© 2016 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

UN SDGs

This output contributes to the following UN Sustainable Development Goals (SDGs)

SDG 7 Affordable and Clean Energy

Keywords

bimesitylenes
hole-transporting materials
perovskite solar cell
stability
twisted structure

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10.1002/cssc.201501392

Cite this

Lin, Y. D., Ke, B. Y., Lee, K. M., Chang, S. H., Wang, K. H., Huang, S. H., Wu, C. G., Chou, P. T., Jhulki, S., Moorthy, J. N., Chang, Y. J., Liau, K. L., Chung, H. C., Liu, C. Y., Sun, S. S., & Chow, T. J. (2016). Hole-Transporting Materials Based on Twisted Bimesitylenes for Stable Perovskite Solar Cells with High Efficiency. ChemSusChem, 9(3), 274-279. https://doi.org/10.1002/cssc.201501392

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title = "Hole-Transporting Materials Based on Twisted Bimesitylenes for Stable Perovskite Solar Cells with High Efficiency",

abstract = "A new class of hole-transport materials (HTMs) based on the bimesitylene core designed for mesoporous perovskite solar cells is introduced. Devices fabricated using two of these derivatives yield higher open-circuit voltage values than the commonly used spiro-OMeTAD. Power conversion efficiency (PCE) values of up to 12.11 \% are obtained in perovskite-based devices using these new HTMs. The stability of the device made using the highest performing HTM (P1) is improved compared with spiro-OMeTAD as evidenced through long-term stability tests over 1000h.",

keywords = "bimesitylenes, hole-transporting materials, perovskite solar cell, stability, twisted structure",

author = "Lin, \{Yan Duo\} and Ke, \{Bo Yu\} and Lee, \{Kun Mu\} and Chang, \{Sheng Hsiung\} and Wang, \{Kai Hung\} and Huang, \{Shih Han\} and Wu, \{Chun Guey\} and Chou, \{Po Ting\} and Samik Jhulki and Moorthy, \{Jarugu Narasimha\} and Chang, \{Yuan Jay\} and Liau, \{Kang Ling\} and Chung, \{Hsin Cheng\} and Liu, \{Ching Yang\} and Sun, \{Shih Sheng\} and Chow, \{Tahsin J.\}",

note = "Publisher Copyright: {\textcopyright} 2016 WILEY-VCH Verlag GmbH \& Co. KGaA, Weinheim.",

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doi = "10.1002/cssc.201501392",

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AU - Lin, Yan Duo

AU - Ke, Bo Yu

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AU - Wang, Kai Hung

AU - Huang, Shih Han

AU - Wu, Chun Guey

AU - Chou, Po Ting

AU - Jhulki, Samik

AU - Moorthy, Jarugu Narasimha

AU - Chang, Yuan Jay

AU - Liau, Kang Ling

AU - Chung, Hsin Cheng

AU - Liu, Ching Yang

AU - Sun, Shih Sheng

AU - Chow, Tahsin J.

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N2 - A new class of hole-transport materials (HTMs) based on the bimesitylene core designed for mesoporous perovskite solar cells is introduced. Devices fabricated using two of these derivatives yield higher open-circuit voltage values than the commonly used spiro-OMeTAD. Power conversion efficiency (PCE) values of up to 12.11 % are obtained in perovskite-based devices using these new HTMs. The stability of the device made using the highest performing HTM (P1) is improved compared with spiro-OMeTAD as evidenced through long-term stability tests over 1000h.

AB - A new class of hole-transport materials (HTMs) based on the bimesitylene core designed for mesoporous perovskite solar cells is introduced. Devices fabricated using two of these derivatives yield higher open-circuit voltage values than the commonly used spiro-OMeTAD. Power conversion efficiency (PCE) values of up to 12.11 % are obtained in perovskite-based devices using these new HTMs. The stability of the device made using the highest performing HTM (P1) is improved compared with spiro-OMeTAD as evidenced through long-term stability tests over 1000h.

KW - bimesitylenes

KW - hole-transporting materials

KW - perovskite solar cell

KW - stability

KW - twisted structure

UR - https://www.scopus.com/pages/publications/84958979863

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JO - ChemSusChem

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IS - 3

ER -

Hole-Transporting Materials Based on Twisted Bimesitylenes for Stable Perovskite Solar Cells with High Efficiency

Abstract

Bibliographical note

UN SDGs

Keywords

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