TY - JOUR
T1 - Lipase-catalyzed hydrolytic resolution of trans-2-(3,4-difluorophenyl)cyclopropyl azolides, a key building block for Ticagrelor synthesis
AU - Wang, Xin Yu
AU - Liu, Jia Xin
AU - Tsai, Shau Wei
N1 - Publisher Copyright:
© 2019 Taiwan Institute of Chemical Engineers
PY - 2019/4
Y1 - 2019/4
N2 - Ticagrelor as a platelet aggregation antagonist can be prepared from (1R,2S)-2-(3,4-diflurophenyl)cyclopropan-1-amine that is converted from (1R,2R)-2-(3,4-diflurophenyl)cyclopropane-1-carboxylic acid ((1R,2R)-DFPCPCA)) via Curtius or Hofmann rearrangement. In this work, an efficient hydrolytic resolution process for the preparation of (1R,2R)-DFPCPCA from trans-2-(3,4-diflurophenyl)cyclopropyl 1,2,4-azolide via an immobilized Candida antarctica lipase B (CALB) in methyl tert‑butyl ether was developed. Quantitative improvements of the enzyme activity and enantioselectivity, i.e., k 2RR K mRR − 1 = 5.512 L/h g and E trans = 197, at 45 °C were obtained. Insights into CALB performances via kinetic and thermodynamic analysis were then addressed and compared with those by using trans-2-phenylcyclopropyl 1,2,4-azolide as the substrate, and demonstrated the prospect of present resolution process for synthesizing other optically pure 2-phenylcyclopropane-1-carboxylic acids containing derivatives in the phenyl subunit in the future.
AB - Ticagrelor as a platelet aggregation antagonist can be prepared from (1R,2S)-2-(3,4-diflurophenyl)cyclopropan-1-amine that is converted from (1R,2R)-2-(3,4-diflurophenyl)cyclopropane-1-carboxylic acid ((1R,2R)-DFPCPCA)) via Curtius or Hofmann rearrangement. In this work, an efficient hydrolytic resolution process for the preparation of (1R,2R)-DFPCPCA from trans-2-(3,4-diflurophenyl)cyclopropyl 1,2,4-azolide via an immobilized Candida antarctica lipase B (CALB) in methyl tert‑butyl ether was developed. Quantitative improvements of the enzyme activity and enantioselectivity, i.e., k 2RR K mRR − 1 = 5.512 L/h g and E trans = 197, at 45 °C were obtained. Insights into CALB performances via kinetic and thermodynamic analysis were then addressed and compared with those by using trans-2-phenylcyclopropyl 1,2,4-azolide as the substrate, and demonstrated the prospect of present resolution process for synthesizing other optically pure 2-phenylcyclopropane-1-carboxylic acids containing derivatives in the phenyl subunit in the future.
KW - Azolides
KW - Hydrolytic resolution
KW - Kinetic and thermodynamic analysis
KW - Lipase
UR - https://www.scopus.com/pages/publications/85062230532
U2 - 10.1016/j.jtice.2019.02.026
DO - 10.1016/j.jtice.2019.02.026
M3 - 文章
AN - SCOPUS:85062230532
SN - 1876-1070
VL - 97
SP - 112
EP - 118
JO - Journal of the Taiwan Institute of Chemical Engineers
JF - Journal of the Taiwan Institute of Chemical Engineers
ER -