USE OF CARBON DIOXIDE AS A HYDROGEN ACCEPTOR IN THE DEHYDROGENATION OF ALKANES.

  • Dale B. Fox*
  • , Emerson H. Lee
  • , Min Hon Rei
  • *Corresponding author for this work

Research output: Contribution to journalConference articlepeer-review

2 Scopus citations

Abstract

Standard catalytic dehydrogenation of alkanes to form olefins has a number of undesirable features as a commercial process. For example, the usual dehydrogenation catalyst such as Cr//2O//3/Al//2O//3 rapidly cokes and deactivates under typical operating conditions. This catalyst may be regenerated with air in a fixed bed or recirculating bed, but the related equipment necessary for this requires an undesirably large capital investment for a commercial plant. Oxidative dehydrogenation is an obvious possibility, but it is difficult to achieve high catalytic selectivity from paraffins to desired products when air or oxygen is used. As an alternative to these processes, carbon dioxide was investigated as an exhaust to effect dehydrogenation and coke removal.

Original languageEnglish
Pages (from-to)b7-b12
JournalAmerican Chemical Society, Division of Petroleum Chemistry, Preprints
Volume17
Issue number2
StatePublished - 1972
EventPetroleum Preprints Presented at the 163rd and 164th ACS National Meetings -
Duration: 09 04 197214 04 1972

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